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Eunmi Chae

Korea University · Physics and Astronomy

About the Lab

Professor Eunmi Chae's research lab specializes in the quantum control of ultracold molecules, focusing on laser cooling, trapping, and coherent manipulation of diatomic molecules for quantum information science. The lab develops advanced techniques such as rf-modulated magneto-optical traps, optical tweezer arrays, and microwave-assisted optical cycling to achieve long-lived molecular qubits and entangled states. Key achievements include the demonstration of dipolar spin-exchange interactions, Bell state preparation, and record coherence times for molecular rotational qubits. The lab also pioneers methods for cooling complex molecules with challenging energy level structures, enabling new pathways for quantum simulation and quantum computing with polar molecules.

ultracold moleculesquantum informationoptical tweezersmolecular qubitsquantum simulation

Research Overview

Papers
65
Total Citations
1,035
Papers (5y)
25
Primary Field
Physics and Astronomy

Research Output Trend

Figures are computed from collected data and may differ slightly.

Publications per year (5y)
25total
2022
2023
2024
2025
2026
Citations per year (5y)
258total
20222023202420252026

Selected Papers

15
1
Article|239 citations·2017
Radio Frequency Magneto-Optical Trapping of CaF with High Density
Loïc Anderegg, Benjamin L. Augenbraun, Eunmi Chae, Boerge Hemmerling, Nicholas R. Hutzler, Aakash Ravi, Alejandra Collopy, Jun Ye, Wolfgang Ketterle, John M. Doyle
SJR Q1Physical Review LettersOA

We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and either rf modulated or dc magnetic fields. The rf magneto-optical trap (MOT) confines 1.0(3)×10^{5} CaF molecules at a density of 7(3)×10^{6} cm^{-3}, which is an order of magnitude greater than previous molecular MOTs. Near Doppler-limited temperatures of 340(20) μK are attained. The achieved density enables future work to directly load optical tweezers and create optical arra

Atomic and Molecular Physics, and OpticsPhysics and Astronomy
2
Article|153 citations·2021
of microwave shielding of ultracold molecules
Loïc Anderegg, Sean Burchesky, Yicheng Bao, Scarlett S. Yu, Tijs Karman, Eunmi Chae, Wolfgang Ketterle, John M. Doyle
Radboud Repository (Radboud University)

\n Contains fulltext :\n 236517.pdf (Publisher’s version ) (Open Access)\n

Atomic and Molecular Physics, and OpticsPhysics and Astronomy
3
Article|124 citations·2023
Dipolar spin-exchange and entanglement between molecules in an optical tweezer array
Yicheng Bao, Scarlett S. Yu, Loïc Anderegg, Eunmi Chae, Wolfgang Ketterle, Kang-Kuen Ni, John M. Doyle
SJR Q1ScienceOA

Ultracold polar molecules are promising candidate qubits for quantum computing and quantum simulations. Their long-lived molecular rotational states form robust qubits, and the long-range dipolar interaction between molecules provides quantum entanglement. In this work, we demonstrate dipolar spin-exchange interactions between single calcium monofluoride (CaF) molecules trapped in an optical tweezer array. We realized the spin-[Formula: see text] quantum XY model by encoding an effective spin-[F

Atomic and Molecular Physics, and OpticsPhysics and Astronomy
4
Article|103 citations·2015
Rotational State Microwave Mixing for Laser Cooling of Complex Diatomic Molecules
Mark Yeo, Matthew T. Hummon, Alejandra Collopy, Bo Yan, Boerge Hemmerling, Eunmi Chae, John M. Doyle, Jun Ye
SJR Q1Physical Review LettersOA

We demonstrate the mixing of rotational states in the ground electronic state using microwave radiation to enhance optical cycling in the molecule yttrium (II) monoxide (YO). This mixing technique is used in conjunction with a frequency modulated and chirped continuous wave laser to slow longitudinally a cryogenic buffer-gas beam of YO. We generate a flux of YO below 10 m/s, directly loadable into a three-dimensional magneto-optical trap. This technique opens the door for laser cooling of diatom

Atomic and Molecular Physics, and OpticsPhysics and Astronomy
5
Article|100 citations·2011
Transition to a Bose–Einstein condensate and relaxation explosion of excitons at sub-Kelvin temperatures
Kosuke Yoshioka, Eunmi Chae, Makoto Kuwata‐Gonokami
SJR Q1Nature CommunicationsOA

Quasiparticles in quantum many-body systems have essential roles in modern physical problems. Bose–Einstein condensation (BEC) of excitons in semiconductors is one of the unobserved quantum statistical phenomena predicted in the photoexcited quasiparticles in many-body electrons. In particular, para-excitons in cuprous oxide have been studied for decades because the decoupling from the radiation field makes the coherent ensemble a purely matter-like wave. However, BEC has turned out to be hard t

Atomic and Molecular Physics, and OpticsPhysics and Astronomy
6
Article|83 citations·2021
Rotational Coherence Times of Polar Molecules in Optical Tweezers
Sean Burchesky, Loïc Anderegg, Yicheng Bao, Scarlett S. Yu, Eunmi Chae, Wolfgang Ketterle, Kang-Kuen Ni, John M. Doyle
SJR Q1Physical Review LettersOA

Qubit coherence times are critical to the performance of any robust quantum computing platform. For quantum information processing using arrays of polar molecules, a key performance parameter is the molecular rotational coherence time. We report a 93(7) ms coherence time for rotational state qubits of laser cooled CaF molecules in optical tweezer traps, over an order of magnitude longer than previous systems. Inhomogeneous broadening due to the differential polarizability between the qubit state

Atomic and Molecular Physics, and OpticsPhysics and Astronomy
7
Article|62 citations·2024
An elementary review on basic principles and developments of qubits for quantum computing
Eunmi Chae, Joonhee Choi, Junki Kim
SJR Q1Nano ConvergenceOA

An elementary review on principles of qubits and their prospects for quantum computing is provided. Due to its rapid development, quantum computing has attracted considerable attention as a core technology for the next generation and has demonstrated its potential in simulations of exotic materials, molecular structures, and theoretical computer science. To achieve fully error-corrected quantum computers, building a logical qubit from multiple physical qubits is crucial. The number of physical q

Artificial IntelligenceComputer Science
8
Article|30 citations·2014
Buffer gas loaded magneto-optical traps for Yb, Tm, Er and Ho
Boerge Hemmerling, Garrett Drayna, Eunmi Chae, Aakash Ravi, John M. Doyle
SJR Q1New Journal of PhysicsOA

Direct loading of lanthanide atoms into magneto-optical traps (MOTs) from a very slow cryogenic buffer gas beam source is achieved, without the need for laser slowing. The beam source has an average forward velocity of 60--70 m s 1 and a velocity half-width of -35 m s 1 , which allows for direct MOT loading of Yb, Tm, Er and Ho. Residual helium background gas originating from the beam results in a maximum trap lifetime of about 80 ms (with Yb). The addition of a single-frequency slowing laser ap

Atomic and Molecular Physics, and OpticsPhysics and Astronomy
9
Article|26 citations·2002
STACEE Observations of Markarian 421 during an Extended Gamma-Ray Outburst
L. M. Boone, J. A. Hinton, D. Bramel, Eunmi Chae, C. E. Covault, P. Fortin, D. M. Gingrich, D. Hanna, R. Mukherjee, Carmen Mueller, R. A. Ong, K. Ragan
SJR Q1The Astrophysical JournalOA

The active galaxy Markarian 421 underwent a substantial outburst in early 2001. Between January and May of that year, the STACEE detector was used to observe the source in gamma-rays between the energies of 50 and 500 GeV. These observations represent the lowest energy gamma-ray detection of this outburst by a ground-based experiment. Here we present results from these observations, which indicate an average integral gamma-ray flux of (8.0 +/- 0.7 +/- 1.5)x10^-10 1/cm^2/s. above 140 GeV. We also

Nuclear and High Energy PhysicsPhysics and Astronomy
10
Article|17 citations·2021
Compact green Ti:sapphire astro-comb with a 43 GHz repetition frequency
Eunmi Chae, Eiji Kambe, Kentaro Motohara, Hideyuki Izumiura, Mamoru Doi, Kosuke Yoshioka
SJR Q2Journal of the Optical Society of America BOA

A compact green astro-comb with a 43 GHz repetition rate is developed based on a Ti:sapphire optical frequency comb (OFC) and a mode-selecting cavity. The OFC’s large repetition rate of 1.6 GHz eases the requirements for the mode-selecting cavity. Unnecessary frequency modes of the OFC are suppressed down to <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mn>5</mml:mn> <mml:mo>×</mml:mo> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:msup> <mml:mn>10</mml:mn> <mml:mrow c

Atomic and Molecular Physics, and OpticsPhysics and Astronomy
11
Article|15 citations·2024
Raman Sideband Cooling of Molecules in an Optical Tweezer Array to the 3D Motional Ground State
Yicheng Bao, Scarlett S. Yu, Jiaqi You, Loïc Anderegg, Eunmi Chae, Wolfgang Ketterle, Kang-Kuen Ni, John M. Doyle
SJR Q1Physical Review XOA

Ultracold polar molecules are promising for quantum information processing and searches for physics beyond the standard model. Laser cooling to ultracold temperatures is an established technique for trapped diatomic and triatomic molecules. Further cooling of the molecules to near the motional ground state is crucial for reducing various dephasings in quantum and precision applications. In this work, we demonstrate Raman sideband cooling (RSC) of CaF molecules in optical tweezers to near their m

Atomic and Molecular Physics, and OpticsPhysics and Astronomy
12
Article|14 citations·2022
Fast optical transport of ultracold molecules over long distances
Yicheng Bao, Scarlett S. Yu, Loïc Anderegg, Sean Burchesky, Derick Gonzalez-Acevedo, Eunmi Chae, Wolfgang Ketterle, Kang-Kuen Ni, John M. Doyle
SJR Q1New Journal of PhysicsOA

Abstract Optically trapped laser-cooled polar molecules hold promise for new science and technology in quantum information and quantum simulation. Large numerical aperture optical access and long trap lifetimes are needed for many studies, but these requirements are challenging to achieve in a magneto-optical trap (MOT) vacuum chamber that is connected to a cryogenic buffer gas beam source, as is the case for all molecule laser cooling experiments so far. Long distance transport of molecules gre

Atomic and Molecular Physics, and OpticsPhysics and Astronomy
13
Preprint|13 citations·2022
Dipolar spin-exchange and entanglement between molecules in an optical tweezer array
Yicheng K. Bao, Scarlett S. Yu, Loïc Anderegg, Eunmi Chae, Wolfgang Ketterle, Kang-Kuen Ni, John M. Doyle
arXiv (Cornell University)OA

Due to their intrinsic electric dipole moments and rich internal structure, ultracold polar molecules are promising candidate qubits for quantum computing and for a wide range of quantum simulations. Their long-lived molecular rotational states form robust qubits while the long-range dipolar interaction between molecules provides quantum entanglement. Using a molecular optical tweezer array, single molecules can be moved and separately addressed for qubit operations using optical and microwave f

Atomic and Molecular Physics, and OpticsPhysics and Astronomy
14
Article|9 citations·2024
PTAA‐infiltrated thin‐walled carbon nanotube electrode with hidden encapsulation for perovskite solar cells
Eunmi Chae, You‐Hyun Seo, Bong Joo Kang, Jin Ho Oh, Yeonsu Jung, Jinho Jang, Tae‐Hoon Kim, Yong‐Ryun Jo, Dong Jun Kim, Taek‐Soo Kim, Sang Hyuk Im, Sae Jin Sung
SJR Q1EcoMatOA

Abstract In perovskite solar cells (PSCs), expensive gold or silver metal has traditionally been utilized as the rear electrode for highly efficient performance. In this context, carbon nanotube (CNT) electrodes have been considered promising rear electrodes because of their excellent electrical conductivity, mechanical strength, and chemical stability in PSCs. Despite these favorable characteristics, concerns have been raised about the power conversion efficiency (PCE) and stability of PSCs bas

Electrical and Electronic EngineeringEngineering
15
Article|7 citations·2023
Laser cooling of molecules
Eunmi Chae
SJR Q3Journal of the Korean Physical SocietyOA
Atomic and Molecular Physics, and OpticsPhysics and Astronomy

Research Areas

Atomic and Molecular Physics, and OpticsElectrical and Electronic EngineeringNuclear and High Energy PhysicsMaterials ChemistryArtificial IntelligenceBiomedical Engineering

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