Wonyoung Lee

Proton conducting electrochemical cells, especially protonic ceramic fuel cells (PCFCs), are expected to be a breakthrough technology in next-generation energy conversion systems, primarily because of their high proton conductivity and low activation energy below 600 °C.

Cation segregation, particularly Sr segregation, toward a perovskite surface has a significant effect on the performance degradation of a solid oxide cell (solid oxide electrolysis/fuel cell). Among the number of key reasons generating the instability of perovskite oxide, surface-accumulated positively charged defects (oxygen vacancy, Vo··) have been considered as the most crucial drivers in strongly attracting negatively charged defects (SrA – site′) toward the surface. Herein, we demonstrate t

Abstract Direct methane protonic ceramic fuel cells are promising electrochemical devices that address the technical and economic challenges of conventional ceramic fuel cells. However, Ni, a catalyst of protonic ceramic fuel cells exhibits sluggish reaction kinetics for CH 4 conversion and a low tolerance against carbon-coking, limiting its wider applications. Herein, we introduce a self-assembled Ni-Rh bimetallic catalyst that exhibits a significantly high CH 4 conversion and carbon-coking tol

Abstract The low‐temperature (<500 °C) operation of reversible protonic ceramic electrochemical cells (PCECs) is desirable in achieving efficient and sustainable electricity generation, as well as green hydrogen production. However, significant interfacial resistance, which contributes to both ohmic and polarization resistance, remains a hurdle in lowering the operating temperature. In this study, PrBa 0.5 Sr 0.5 Co 1.5 Fe 0.5 O 5+δ (PBSCF) and BaZr 0.4 Ce 0.4 Y 0.1 Yb 0.1 O 3‐δ (BZCYYb) mono

Nano-structured composite electrodes, from a carefully conducted infiltration process, are one of the most promising electrode structures for intermediate temperature solid oxide fuel cells (IT-SOFCs), due to their ability to promote the oxygen reduction reaction (ORR) and enlarge triple phase boundaries (TPBs).

Graphene oxide (GO), which is the oxidized form of graphene, has holes and functional groups on the surface and thus has high potential to be used as an electrochemical transport channel material. In this study, differently modified GO membranes are applied as electrolytes of proton exchange membrane fuel cells (PEMFCs) with controlled carbon/oxygen ratios. The critical and desired properties of the electrolyte, such as electron conductivity, proton conductivity, interfacial reactivity, and cell

A novel thin-film coating technique using a gelatin-based GDC precursor solution was developed for dense and smooth 2D layers achieving excellent chemical stability.

Engineering the defect chemistry at the interface between the electrolyte and the electrode is crucial to facilitate oxygen reduction reaction, thereby improve the electrochemical performance of intermediate temperature solid oxide fuel cells.