Dongwook Go

We show theoretically that both the intrinsic spin Hall effect (SHE) and orbital Hall effect (OHE) can arise in centrosymmetric systems through momentum-space orbital texture, which is ubiquitous even in centrosymmetric systems unlike spin texture. The OHE occurs even without spin-orbit coupling (SOC) and is converted into the SHE through SOC. The resulting spin Hall conductivity is large (comparable to that of Pt) but depends on the SOC strength in a nonmonotonic way. This mechanism is stable a

In solids, electronic Bloch states are formed by atomic orbitals. While it is natural to expect that orbital composition and information about Bloch states can be manipulated and transported, in analogy to the spin degree of freedom extensively studied in past decades, it has been assumed that orbital quenching by the crystal field prevents significant dynamics of orbital degrees of freedom. However, recent studies reveal that an orbital current, given by the flow of electrons with a finite orbi

Abstract As the inversion symmetry is broken at a surface, spin-orbit interaction gives rise to spin-dependent energy shifts – a phenomenon which is known as the spin Rashba effect. Recently, it has been recognized that an orbital counterpart of the spin Rashba effect – the orbital Rashba effect – can be realized at surfaces even without spin-orbit coupling. Here, we propose a mechanism for the orbital Rashba effect based on sp orbital hybridization, which ultimately leads to the electric polari

Recent experimental observation of an unexpectedly large current-induced spin-orbit torque in surface oxidized Cu on top of a ferromagnet pointed to a possibly prominent role of the orbital Rashba effect (ORE) in this system. Here, we use first principles methods to investigate the ORE in a system of oxygen monolayer deposited on top of a Cu(111) film. We show that surface oxidization of the Cu film leads to a gigantic enhancement of the ORE near the Fermi energy. The resulting chiral orbital te

While it is often assumed that the orbital response is suppressed and short ranged due to strong crystal field potential and orbital quenching, we show that the orbital response can be remarkably long ranged in ferromagnets. In a bilayer consisting of a nonmagnet and a ferromagnet, spin injection from the interface results in spin accumulation and torque in the ferromagnet, which rapidly oscillate and decay by spin dephasing. In contrast, even when an external electric field is applied only on t

In the emerging field of orbitronics, the orbital Hall effect stands out as one of the most important transport phenomena of orbital angular momentum. Here, the authors present a highly efficient and accurate first-principles method to compute the orbital Hall effect by Wannier interpolation and point out the crucial role of the anomalous position for the gauge-covariant description. The work guides the ongoing experimental efforts on the quantitative measurement of orbital currents.

We propose a concept of noncollinear spin current, whose spin polarization varies in space even in nonmagnetic crystals. While it is commonly assumed that the spin polarization of the spin Hall current is uniform, asymmetric local crystal potential generally allows the spin polarization to be noncollinear in space. Based on microscopic considerations, we demonstrate that such noncollinear spin Hall currents can be observed, for example, in layered Kagome Mn_{3}X (X=Ge, Sn) compounds. Moreover, b

When the inversion symmetry is broken at a surface, spin-orbit interaction gives rise to spin-dependent energy shifts - a phenomenon which is known as the spin Rashba effect. Recently, it has been recognized that an orbital counterpart of the spin Rashba effect - the orbital Rashba effect - can be realized at surfaces even without spin- orbit coupling. Here, we propose a mechanism for the orbital Rashba effect based on sp orbital hybridization, which ultimately leads to the electric polarization

We show that dynamics of the magnetization in ferromagnets can pump orbital angular momentum, a phenomenon we refer to as orbital pumping. This is the reciprocal phenomenon to orbital torque that induces magnetization dynamics by the orbital angular momentum in nonequilibrium. The orbital pumping is analogous to the spin pumping established in spintronics, but it requires spin-orbit coupling for the orbital angular momentum to interact with magnetization. We develop a formalism that describes th

Chirality is ubiquitous in nature and manifests in a wide range of phenomena including chemical reactions, biological processes, and quantum transport of electrons. In quantum materials, the chirality of fermions, given by the relative directions between the electron spin and momentum, is connected to the band topology of electronic states. This study shows that in structurally chiral materials like CoSi, the orbital angular momentum (OAM) serves as the main driver of a nontrivial band topology

We show that dynamics of the magnetization in ferromagnets can pump the orbital angular momentum, which we denote by orbital pumping. This is the reciprocal phenomenon to the orbital torque that induces magnetization dynamics by the orbital angular momentum in non-equilibrium. The orbital pumping is analogous to the spin pumping established in spintronics but requires the spin-orbit coupling for the orbital angular momentum to interact with the magnetization. We develop a formalism that describe

The position operator in a Bloch representation acquires a gauge correction in the momentum space on top of the canonical position, which is called the anomalous position. We show that the anomalous position is generally orbital-dependent and thus plays a crucial role in the description of the intrinsic orbital Hall effect in terms of Wannier basis. We demonstrate this from the first-principles calculation of orbital Hall conductivities of transition metals by Wannier interpolation. Our results

Efficient manipulation of magnetization by electrical current is a key aim in spintronics. The state-of-the-art theories and experiments in spintronics show that harnessing non-equilibrium orbital angular momentum can significantly enhance the efficiency due to novel torques. Devices are based on environment-friendly materials, which has been difficult to achieve by the mechanisms based on spin only, and this has also kickstarted a new emerging field of research: orbitronics.

While it is often assumed that the orbital response is suppressed and short-ranged due to strong crystal field potential and orbital quenching, we show that the orbital magnetoelectric response can be remarkably long-ranged in ferromagnets. In a bilayer consisting of a nonmagnet and a ferromagnet, spin injection from the interface results in spin accumulation and torque in the ferromagnet, which rapidly oscillate and decay by spin dephasing. In contrast, we find that even when an external electr