Y. Kondo

Submicron organic aerosol was measured simultaneously with an Aerodyne aerosol mass spectrometer (AMS) and a particle‐into‐liquid sampler (PILS) capable of measuring water‐soluble organic carbon (WSOC) during the winter and summer of 2004 in Tokyo. Both techniques are being used to investigate the formation of secondary organic aerosol (SOA), and the combined data sets provide unique insights. In summer, about 80% (40–65%) of organic aerosols were oxygenated when scaled by total (carbon) mass co

Reliable assessment of the impact of aerosols emitted from boreal forest fires on the Arctic climate necessitates improved understanding of emissions and the microphysical properties of carbonaceous (black carbon (BC) and organic aerosols (OA)) and inorganic aerosols. The size distributions of BC were measured by an SP2 based on the laser-induced incandescence technique on board the DC-8 aircraft during the NASA ARCTAS campaign. Aircraft sampling was made in fresh plumes strongly impacted by wil

In this study, we show that black carbon (BC) mass concentrations measured by different techniques are consistent and traceable. First, we present the volatilities of 13 organic compounds passed through a heated inlet. These data were used to quantify the interference of organic aerosols on the BC measurement techniques. The masses of the refractory particles that incandesce (m*ref) were used to calibrate BC mass measured by a single-particle soot photometer (SP2), which uses laser-induced incan

Mass concentrations of elemental carbon (EC) in fine mode and mixing ratios of carbon monoxide (CO) were measured at the University of Tokyo campus in Tokyo in different seasons in 2003–2005. Measurements of EC were made using a semicontinuous thermal‐optical analyzer. The mass concentrations of nonvolatile aerosol measured by the calibrated scanning mobility particle sizer combined with a heated inlet agreed with the independent EC measurements with a systematic difference of about 4%, demonstr

Abstract. Fires and the aerosols that they emit impact air quality, health, and climate, but the abundance and properties of carbonaceous aerosol (both black carbon and organic carbon) from biomass burning (BB) remain uncertain and poorly constrained. We aim to explore the uncertainties associated with fire emissions and their air quality and radiative impacts from underlying dry matter consumed and emissions factors. To investigate this, we compare model simulations from a global chemical trans

In principle, mass concentrations of black carbon (BC) (M BC) can be estimated by the measurement of the light absorption coefficient of BC. Filter-based methods, which quantify the absorption coefficient (b abs) from the change in transmission through a filter loaded with particles, have been widely used to measure M BC. However, reliable determination of M BC has been very difficult because of the large variability in the mass absorption cross section (C abs), which is the conversion factor fr