Chang‐Ha Lee
Yonsei University · 工学
研究室紹介
Professor Chang-Ha Lee's research lab specializes in adsorption science and separation processes, with a strong focus on the development and optimization of advanced adsorbents—such as zeolites, activated carbon, and carbon molecular sieves—for gas and vapor separation. The lab investigates equilibrium and dynamic adsorption behaviors, particularly for CO₂, CH₄, H₂, and water vapor, using both experimental and theoretical approaches. Key research directions include pressure swing adsorption (PSA) processes for hydrogen purification, landfill gas upgrading, and carbon dioxide capture, with an emphasis on accurate modeling that accounts for heat effects and concentration-dependent mass transfer.
Research Overview
Research Output Trend
Figures are computed from collected data and may differ slightly.
Selected Papers
15The adsorption equilibria of CO 2 on zeolite 13X and zeolite X/activated carbon composite (Zeocarbon) were measured by a static volumetric method. The equilibrium experiments were conducted at (273.15, 293.15, 313.15, 333.15, and 353.15) K and at pressures up to 102.0 kPa for zeolite 13X and 99.7 kPa for Zeocarbon. The experimental data obtained were correlated by the Toth, UNILAN, and Sips models, which are generally used for microporous adsorbents such as zeolites and activated carbon. The iso
The adsorption equilibria of water vapor on zeolite 3A, zeolite 13X, and dealuminated Y zeolite (DAY) were measured using a volumetric method. Equilibrium experiments were conducted at 293.15, 303.15, and 313.15 K and at relative pressure ( P / P s ) up to 0.95. Experimental data were correlated using Aranovich–Donohue and Frenkel–Halsey–Hill models, using Langmuir, Toth, UNILAN, and Sips isotherms.
The adsorption equilibria of water vapor on Al 2 O 3, zeolite 13X, and a zeolite X/activated carbon composite (Zeocarbon) were measured by a static volumetric method. The equilibrium experiments were conducted at (293.2, 313.2, 333.1, and 353.1) K and pressures up to 2.1 kPa for Al 2 O 3 and 2.3 kPa for zeolite 13X and Zeocarbon, respectively. The experimental data obtained were correlated by the Aranovich and Donohue (A−D) and n -layer BET models.
A study on a two-bed six-step pressure swing adsorption (PSA) process using zeolite 5A was performed experimentally and theoretically for bulk separation of H 2 /CO and H 2 /CH 4 systems (70/30 vol %) as major components in coke oven gas. When the pressure is cycled between 1 and 11 atm at ambient temperatures, 70% H 2 in the feed could be concentrated to 99.99% in the product with a recovery of 75.87% in the H 2 /CO mixture and 80.38% in the H 2 /CH 4 mixture. The effects of adsorption pressure
Adsorption characteristics in a layered bed packed with activated carbon and zeolite 5A were studied experimentally and theoretically through the breakthrough experiments of binary (H 2 /CO, H 2 /CH 4, H 2 /CO 2 ), ternary (H 2 /CH 4 /CO), and five-component (H 2 /CH 4 /CO/N 2 /CO 2 ) systems. The effects of adsorption pressure, feed flow rate, and carbon-to-zeolite ratio on the breakthrough curve in a layered bed were observed. Breakthrough curves in all of the mixtures showed tailing due to te